So we have the base 16 allomantic (a) metals that are also used in feruchemy and hemalurgy (f and h). Following this, if any more a metals are found, then they will be used in f and h too. However, this can be reversed. If a=f=h, then if more h or f metals are found, they will be used in a as well. However, we also have the God metals and their alloys. Since there are 16 base metals, there will probably be another set of 16 per God metal. This means that, for lerasium, atium and harmonium, there is another set of 16. So, there must be 64 metals, plus their alloys. However, since lerasium makes you a Mistborn and atium can steal any power or attribute better than any other metal, harmonium will most probably be able to gift feruchemy to anyone who taps/stores it. So, in total, there must be 67 metals, used for a, f and h